Electrochemical synthesis of magnetite and maghemite nanoparticles using dissymmetric potential pulses
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Magnetic iron oxide nanoparticles of controlled size distribution were electrochemically synthesized applying a dissymmetric pattern of potential pulses to iron-based electrodes in aqueous media. The best pattern was determined through a design of experiments based on a previous voltammetric study. The applied method conveys an optimization of previous methods which employed direct or symmetric alternate potentials. XRD results indicate that magnetite phase is favored to anodic potentials larger -0.2 V versus SSE. TEM images show quasi spherical particles with size ranging from 10 to 50 nm, depending on the synthesis conditions, which agrees with size estimated from diffractograms. EDS indicate that the electrolyte is not totally eliminated by washing although its content is lower than 1 %25. © 2012 Springer Science Business Media B.V.
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Magnetic iron oxide nanoparticles of controlled size distribution were electrochemically synthesized applying a dissymmetric pattern of potential pulses to iron-based electrodes in aqueous media. The best pattern was determined through a design of experiments based on a previous voltammetric study. The applied method conveys an optimization of previous methods which employed direct or symmetric alternate potentials. XRD results indicate that magnetite phase is favored to anodic potentials larger -0.2 V versus SSE. TEM images show quasi spherical particles with size ranging from 10 to 50 nm, depending on the synthesis conditions, which agrees with size estimated from diffractograms. EDS indicate that the electrolyte is not totally eliminated by washing although its content is lower than 1 %25. © 2012 Springer Science%2bBusiness Media B.V.
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Electrochemical synthesis; Magnetite nanoparticles; Potential pulses Design of experiments; Electrolytes; Iron oxides; Magnetic nanoparticles; Magnetite; Magnetite nanoparticles; Anodic potentials; Electrochemical synthesis; Maghemite nanoparticle; Magnetic iron oxide nanoparticles; Potential pulse; Spherical particle; Synthesis conditions; Voltammetric studies; Synthesis (chemical); ferric oxide; magnetite; nanoparticle; article; electric potential; electrochemical analysis; electrode; particle size; potentiometry; priority journal; X ray diffraction
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