Structural study, photoluminescence, and photocatalytic activity of semiconducting BaZrO3:Bi nanocrystals
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Wide band gap nanocrystalline bismuth doped barium zirconate is synthesized by a facile hydrothermal method at 100 °C. The obtained cubic perovskites are characterized by powder X-ray diffraction (XRD), UV-VIS diffuse reflectance spectroscopy, photoluminescence (PL) spectroscopy, and photocatalytic activity. The estimated band gap in the 2.4-4.9 eV range, depending on Bi concentration, suggests nanocrystalline BaZrO3:Bi as a useful visible-light activated photocatalyst under excitation wavelengths <800 nm. Displacement of main XRD pattern peaks suggest that bismuth ion mostly substitutes into Zr 4 sites within the BaZrO3 host lattice. It is found that BaZrO3:Bi decomposes methylene blue (MB) under both UV and visible light irradiation. The photocatalyst efficiency depends strongly on Bi content and induced defects. © 2011 Elsevier B.V.
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Wide band gap nanocrystalline bismuth doped barium zirconate is synthesized by a facile hydrothermal method at 100 °C. The obtained cubic perovskites are characterized by powder X-ray diffraction (XRD), UV-VIS diffuse reflectance spectroscopy, photoluminescence (PL) spectroscopy, and photocatalytic activity. The estimated band gap in the 2.4-4.9 eV range, depending on Bi concentration, suggests nanocrystalline BaZrO3:Bi as a useful visible-light activated photocatalyst under excitation wavelengths <800 nm. Displacement of main XRD pattern peaks suggest that bismuth ion mostly substitutes into Zr 4%2b sites within the BaZrO3 host lattice. It is found that BaZrO3:Bi decomposes methylene blue (MB) under both UV and visible light irradiation. The photocatalyst efficiency depends strongly on Bi content and induced defects. © 2011 Elsevier B.V.
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Barium zirconate; Bismuth; Nanocrystals; Photocatalyst Bismuth ion; Bismuth-doped; Cubic perovskite; Excitation wavelength; Host lattice; Hydrothermal methods; Induced defects; Methylene blue; Nanocrystallines; Photocatalytic activities; Powder X ray diffraction; Structural studies; UV and visible light; UV-Vis diffuse reflectance spectroscopy; Visible light; Wide band gap; XRD patterns; Barium; Bismuth; Energy gap; Light; Nanocrystals; Perovskite; Photocatalysis; Photocatalysts; Photoluminescence; Photoluminescence spectroscopy; X ray diffraction; Zirconium; Barium zirconate
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