Electrochemical sensor for thiourea focused on metallurgical applications of copper
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A simple and reliable device is presented for the direct monitoring of thiourea in copper electrorefinery baths as a tool for reconditioning of industrial baths, and so reducing its environmental impact. For this purpose, a screen-printed graphite electrode is modified with silver nanoparticles (AgNPs) contained in a polyelectrolyte-surfactant matrix. The AgNPs are able to adsorb the thiourea, improving the sensitivity of the electrode toward this analyte, even in the presence of usual additives (Avitone® and glue). The system allows the determination of thiourea in a range of 1-10 mg/L. A coupled electrochemical and IR analysis is proposed to evaluate the involved mechanism. © 2016 Elsevier B.V. All rights reserved.
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Copper electrorefining; Infrared spectroscopy; Silver nanoparticles; Square wave voltammetry; Thiourea; Voltammetry Copper; Electrochemical sensors; Electrodes; Environmental impact; Graphite electrodes; Infrared spectroscopy; Metal nanoparticles; Nanoparticles; Polyelectrolytes; Silver; Voltammetry; Copper electrorefining; Direct monitoring; IR analysis; Metallurgical applications; Screen printed graphite electrodes; Silver nanoparticles; Silver nanoparticles (AgNps); Square wave voltammetry; Thioureas
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