Spin-reorientation transitions in one-dimensional and two-dimensional magnetic nanostructures
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abstract
The magnetic anisotropy energy (MAE) of 3d transition-metal wires, stripes, and films is calculated self-consistently as a function of stripe width and film thickness. The magnetization-reorientation transitions in stripes are determined along the crossover from the mono-atomic one-dimensional chain to the two-dimensional monolayer. It is shown that the MAE oscillates as a function of stripe width and depends strongly on the considered transition metal. The reorientation transitions in Co films deposited on a highly polarizable substrate such as Pd are discussed. A local analysis of the layer-resolved MAEs provides new insights into the off-plane magnetization observed in Pd-capped Co films on Pd(111). The interfaces responsible for the stability of the off-plane easy axis are characterized microscopically. An unexpected internal magnetic structure of the Co-Pd interfaces is revealed in which the magnetic moments and spin-orbit interactions at Pd atoms play a crucial role. The nature of the reorientation transition from perpendicular to in-plane magnetization with increasing film thickness is studied by means of full-vectorial calculations. The existence of a spin-canted phase at intermediate film thickness is demonstrated.
Magnetic nanostructures; Spin-reorientation transitions Ground state; Magnetic fields; Magnetic materials; Magnetic moments; Magnetization; Monolayers; Scanning electron microscopy; Transition metals; Two dimensional; Film thickness; Magnetic anisotropy energy (MAE); Magnetic nanostructures; Spin-reorientation transitions; Nanostructured materials