Energy landscape of colloidal dumbbells in a periodic distribution of light

Using a ray tracing calculation, the energy landscape of dumbbells, made of spherical colloidal particles, interacting with a periodic distribution of light is calculated. As shown previously [E. Sarmiento-Gomez, J. A. Rivera-Moran and J. L. Aruaz-Lara, Soft Matter, 2018, 14, 3684], planar aggregates of spherical particles adopt discrete configurations in such light distribution. Here we focus on the case of colloidal dumbbells both symmetric and asymmetric from an experimental and theoretical point of view. It has been shown that the direct calculation using the ray tracing approximation is in excellent agreement with the experiment in spite of the fact that the particles size and the wavelength of the trapping light are comparable. We also corroborate, at least for the more simple case of a single particle in a parabolic light distribution, that the simple method used here provides the same results as the more complex and general Lorenz-Mie approach giving a more simple yet reliable method for the calculation of the energy landscape of colloidal aggregates in periodic light distributions. © 2019 The Royal Society of Chemistry.

Aggregates; Colloidal aggregates; Discrete configurations; Light distribution; Periodic distribution; Ray tracing calculations; Spherical colloidal particles; Spherical particle; Theoretical points; Ray tracing

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