Synthesis and Evaluation of a Molecularly Imprinted Polymer for the Determination of Metronidazole in Water Samples
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A molecularly imprinted polymer was developed and evaluated for selective determination of metronidazole (MNZ) in wastewater. This was achieved by using sodium methacrylate as monomer, toluene as porogen, ethylene glycol dimethacrylate as crosslinker, azobisisobutyronitrile as initiator and metronidazole as template molecule to generate the selectivity of the polymer for the compound, as well as non-imprinted polymers were synthesized. Two different polymerization approaches were used, bulk and emulsion and the polymers obtained by emulsion presented higher retention percentages the MIP 2-M presented the higher retention (83%25). The performed method, was validated in fortified water, showing linearity from 10 up to 1000 ng/mL; limit of detection and quantification for compound were between 3 and 10 ng/mL, respectively. Finally, the method was applied in samples of a wastewater treatment plant in the city of San Luis Potosí, México, and the concentrations of MNZ in these samples were 84.1–114 ng/mL. © 2017, Springer Science Business Media, LLC, part of Springer Nature.
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A molecularly imprinted polymer was developed and evaluated for selective determination of metronidazole (MNZ) in wastewater. This was achieved by using sodium methacrylate as monomer, toluene as porogen, ethylene glycol dimethacrylate as crosslinker, azobisisobutyronitrile as initiator and metronidazole as template molecule to generate the selectivity of the polymer for the compound, as well as non-imprinted polymers were synthesized. Two different polymerization approaches were used, bulk and emulsion and the polymers obtained by emulsion presented higher retention percentages the MIP 2-M presented the higher retention (83%25). The performed method, was validated in fortified water, showing linearity from 10 up to 1000 ng/mL; limit of detection and quantification for compound were between 3 and 10 ng/mL, respectively. Finally, the method was applied in samples of a wastewater treatment plant in the city of San Luis Potosí, México, and the concentrations of MNZ in these samples were 84.1–114 ng/mL. © 2017, Springer Science%2bBusiness Media, LLC, part of Springer Nature.
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Metronidazole; Molecularly imprinted polymer; Non-imprinted polymer; Wastewater Emulsification; Ethylene; Ethylene glycol; Synthesis (chemical); Wastewater; Azobisisobutyronitrile; Ethylene glycol dimethacrylate; Metronidazole; Molecularly Imprinted Polymer; Non-imprinted polymers; Selective determination; Sodium methacrylates; Wastewater treatment plants; Wastewater treatment; azobis(isobutyronitrile); ethylene glycol dimethacrylate; methacrylic acid; methacrylic acid derivative; metronidazole; nitrile; polymethacrylic acid derivative; toluene; adsorption; analysis; chemistry; limit of detection; Mexico; molecular imprinting; procedures; surface property; synthesis; waste water; water pollutant; Adsorption; Limit of Detection; Methacrylates; Metronidazole; Mexico; Molecular Imprinting; Nitriles; Polymethacrylic Acids; Surface Properties; Toluene; Waste Water; Water Pollutants, Chemical
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