Magnetic quantum coherence effect inNi4 molecular transistors
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We present a theoretical study of electron transport in Ni4 molecular transistors in the presence of Zeeman spin splitting and magnetic quantum coherence (MQC). The Zeeman interaction is extended along the leads which produces gaps in the energy spectrum which allow electron transport with spin polarized along a certain direction. We show that the coherent states in resonance with the spin up or down states in the leads induces an effective coupling between localized spin states and continuum spin states in the single molecule magnet and leads, respectively. We investigate the conductance at zero temperature as a function of the applied bias and magnetic field by means of the Landauer formula, and show that the MQC is responsible for the appearence of resonances. Accordingly, we name them MQC resonances. © 2014 IOP Publishing Ltd.
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Landauer formula; magnetic quantum tunneling; single molecule magnets Electron transport properties; Low temperature engineering; Magnets; Molecules; Quantum theory; Spin dynamics; Electron transport; Landauer formula; Magnetic quantum tunneling; Molecular transistors; Quantum coherence effects; Single-molecule magnet; Zeeman interactions; Zeeman spin splitting; Resonance; metal nanoparticle; nickel; chemical model; chemistry; computer simulation; device failure analysis; electric conductivity; equipment design; magnet; magnetic field; microelectrode; quantum theory; semiconductor; ultrastructure; Computer Simulation; Electric Conductivity; Equipment Design; Equipment Failure Analysis; Magnetic Fields; Magnets; Metal Nanoparticles; Microelectrodes; Models, Chemical; Nickel; Quantum Theory; Transistors, Electronic
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