Epigenetic markers of exposure to polycyclic aromatic hydrocarbons in Mexican brickmakers: A pilot study
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A pilot cross-sectional study was carried out in a group of 39 male brick manufacturers in San Luis Potosi, Mexico to identify epigenetic biomarkers of exposure to polycyclic aromatic hydrocarbons (PAHs). A questionnaire was used to compile the smoking and drinking habits, clinical history, working time, and socioeconomic characteristics of the participants. 1-Hydroxypyrene (1-OHP) levels were measured from urine samples using high-performance liquid chromatography, and genomic DNA was isolated from blood samples for methylation analysis using pyrosequencing. The mean 1-OHP level was 0.18μgg-1 creatinine (range 0.023-1.11), which was below the expected occupational exposure level. After adjusting for potential confounders, the 1-OHP urine concentration was negatively associated with DNA methylation of the interleukin 12 (β=-1.57; 95%25 CI: -2.9 to -0.23; p=0.02) and p53 gene promoters (β=-2.7; 95%25 CI: -5.46-0.06; p=0.055). Suggestive negative associations were also found for the TNF-α gene (β=-3.9; 95%25 CI:-8.28-0.48; p=0.08) and Alu sequences (β=-0.55; 95%25 CI:-1.25-0.16; p=0.12). Although the individual exposures to PAHs as estimated by urinary 1-OHP concentrations were low, changes in specific and global DNA methylation were observed. © 2012 Elsevier Ltd.
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Brickmakers; DNA methylation; Epigenetic markers; Polycyclic aromatic hydrocarbons Alkylation; Aromatization; Brickmaking; DNA; Genes; High performance liquid chromatography; Methylation; Mineral oils; Brickmakers; Cross-sectional study; DNA Methylation; Epigenetic markers; Methylation analysis; Occupational exposure; Polycyclic aromatic hydrocarbons (PAHS); Socioeconomic characteristics; Polycyclic aromatic hydrocarbons; 1 hydroxypyrene; biological marker; gamma interferon; genomic DNA; interleukin 12; polycyclic aromatic hydrocarbon; protein p53; tumor necrosis factor alpha; biomarker; blood; genomics; health risk; liquid chromatography; occupational exposure; PAH; public health; pyrene; questionnaire survey; sampling; smoking; socioeconomic impact; adolescent; adult; aged; article; controlled study; cross-sectional study; DNA determination; DNA isolation; DNA methylation; epigenetics; genetic association; high performance liquid chromatography; human; human experiment; industrial worker; male; Mexico; normal human; occupational exposure; pilot study; promoter region; pyrosequencing; questionnaire; urine level; Mexico [North America]; San Luis Potosi
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